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Titel A size-composition resolved aerosol model for simulating the dynamics of externally mixed particles: SCRAM (v 1.0)
VerfasserIn S. Zhu, K. N. Sartelet, C. Seigneur
Medientyp Artikel
Sprache Englisch
ISSN 1991-959X
Digitales Dokument URL
Erschienen In: Geoscientific Model Development ; 8, no. 6 ; Nr. 8, no. 6 (2015-06-01), S.1595-1612
Datensatznummer 250116398
Publikation (Nr.) Volltext-Dokument vorhandencopernicus.org/gmd-8-1595-2015.pdf
 
Zusammenfassung
The Size-Composition Resolved Aerosol Model (SCRAM) for simulating the dynamics of externally mixed atmospheric particles is presented. This new model classifies aerosols by both composition and size, based on a comprehensive combination of all chemical species and their mass-fraction sections. All three main processes involved in aerosol dynamics (coagulation, condensation/evaporation and nucleation) are included. The model is first validated by comparison with a reference solution and with results of simulations using internally mixed particles. The degree of mixing of particles is investigated in a box model simulation using data representative of air pollution in Greater Paris. The relative influence on the mixing state of the different aerosol processes (condensation/evaporation, coagulation) and of the algorithm used to model condensation/evaporation (bulk equilibrium, dynamic) is studied.
 
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