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Titel Aerosols that form subvisible cirrus at the tropical tropopause
VerfasserIn K. D. Froyd, D. M. Murphy, P. Lawson, D. Baumgardner, R. L. Herman
Medientyp Artikel
Sprache Englisch
ISSN 1680-7316
Digitales Dokument URL
Erschienen In: Atmospheric Chemistry and Physics ; 10, no. 1 ; Nr. 10, no. 1 (2010-01-12), S.209-218
Datensatznummer 250007901
Publikation (Nr.) Volltext-Dokument vorhandencopernicus.org/acp-10-209-2010.pdf
 
Zusammenfassung
The composition of residual particles from evaporated cirrus ice crystals near the tropical tropopause as well as unfrozen aerosols were measured with a single particle mass spectrometer. Subvisible cirrus residuals were predominantly composed of internal mixtures of neutralized sulfate with organic material and were chemically indistinguishable from unfrozen sulfate-organic aerosols. Ice residuals were also similar in size to unfrozen aerosol. Heterogeneous ice nuclei such as mineral dust were not enhanced in these subvisible cirrus residuals. Biomass burning particles were depleted in the residuals. Cloud probe measurements showing low cirrus ice crystal number concentrations were inconsistent with conventional homogeneous freezing. Recent laboratory studies provide heterogeneous nucleation scenarios that may explain tropopause level subvisible cirrus formation.
 
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