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Titel Extinction efficiencies of coated absorbing aerosols measured by cavity ring down aerosol spectrometry
VerfasserIn A. Abo Riziq, M. Trainic, C. Erlick, E. Segre, Y. Rudich
Medientyp Artikel
Sprache Englisch
ISSN 1680-7316
Digitales Dokument URL
Erschienen In: Atmospheric Chemistry and Physics ; 8, no. 6 ; Nr. 8, no. 6 (2008-03-26), S.1823-1833
Datensatznummer 250005942
Publikation (Nr.) Volltext-Dokument vorhandencopernicus.org/acp-8-1823-2008.pdf
 
Zusammenfassung
In this study, we measure the extinction efficiency at 532 nm of absorbing aerosol particles coated with a non-absorbing solid and liquid organic shell with coating thickness varying between 5 and 100 nm using cavity ring down aerosol spectrometry. For this purpose, we use nigrosin, an organic black dye, as a model absorbing core and two non-absorbing organic substances as shells, glutaric acid (GA) and Di-Ethyl-Hexyl-Sebacate (DEHS). The measured behavior of the coated particles is consistent with Mie calculations of core-shell particles. Errors between measured and calculated values for nigrosin coated with GA and DEHS are between 0.5% and 10.5% and between 0.5% and 9%, respectively. However, it is evident that the calculations are in better agreement with the measured results for thinner coatings. Possible reasons for these discrepancies are discussed.
 
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