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Titel Study of the biogenic soil NOx emissions from the Australian desert.
VerfasserIn Penelope Maher, Guergana Guerova, Symeon Koumoutsaris, George Takacs
Konferenz EGU General Assembly 2011
Medientyp Artikel
Sprache Englisch
Digitales Dokument PDF
Erschienen In: GRA - Volume 13 (2011)
Datensatznummer 250049226
 
Zusammenfassung
Nitrogen oxides (NOx) originate from various anthropogenic and natural sources. NOx is a trace gas with broad climate and environmental implications including: acid rain, urban smog, decreasing visibility, soil and stream acidification from leaching and eutrophication. Globally, anthropogenic NOx emissions are well characterised, however, biogenic soil emissions are poorly accounted for. This is partly due the difficulty in performing ground based campaign in remote regions. This study is a first attempt to quantify the soil NOx emissions from the Australian Desert using the synergy between satellite observations from GOME and simulations with global chemistry and transport model GEOS-Chem. Soil NOx emissions from the Australian desert, an area covering 2.5 million km2, are investigated for the year 2000. Inverse modeled NOx emissions were obtained by combining the a priori NOx emissions from GEOS-Chem with GOME and GEOS-Chem tropospheric NO2 columns, to produce a posteriori emission inventory. The total a posterior soil emissions for Australia in 2000 are 0.70 TgN, which accounts for 8% of the global soil NOx emissions. The a posteriori soil emissions from Australia are a factor of 1.7 higher than the a priori. A posteriori soil emissions from the desert in 2000 are 0.31 TgN, which accounts for about 4% of the global soil NOx emissions. Soil emissions from the desert peak during spring (October, November and December) with a posteriori emission of 0.11 TgN, accounting for 1.3% of global soil emissions. The soil NOx emissions from the Australian desert are of the same order of magnitude as the Australian anthropogenic emissions and have the potential to influence air quality in the spring/summer.