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| Titel |
Long-term spatial and temporal variation of CO2 partial pressure in the Yellow River, China |
| VerfasserIn |
L. Ran, X. X. Lu, J. E. Richey, H. Sun, J. Han, R. Yu, S. Liao, Q. Yi |
| Medientyp |
Artikel
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| Sprache |
Englisch
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| ISSN |
1726-4170
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| Digitales Dokument |
URL |
| Erschienen |
In: Biogeosciences ; 12, no. 4 ; Nr. 12, no. 4 (2015-02-16), S.921-932 |
| Datensatznummer |
250117815
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| Publikation (Nr.) |
 copernicus.org/bg-12-921-2015.pdf |
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| Zusammenfassung |
| Carbon transport in river systems is an important
component of the global carbon cycle. Most rivers of the world act as
atmospheric CO2 sources due to high riverine CO2 partial pressure
(pCO2). By determining the pCO2 from alkalinity and pH, we
investigated its spatial and temporal variation in the Yellow River
watershed using historical water chemistry records (1950s–1984) and recent
sampling along the mainstem (2011–2012). Except the headwater region where
the pCO2 was lower than the atmospheric equilibrium (i.e. 380 μatm),
river waters in the remaining watershed were supersaturated with
CO2. The average pCO2 for the watershed was estimated at
2810 ± 1985 μatm, which is 7-fold the atmospheric equilibrium. As
a result of severe soil erosion and dry climate, waters from the Loess
Plateau in the middle reaches had higher pCO2 than that from the upper
and lower reaches. From a seasonal perspective, the pCO2 varied from
about 200 μatm to > 30 000 μatm with higher pCO2
usually occurring in the dry season and lower pCO2 in the wet season (at
73% of the sampling sites), suggesting the dilution effect of water.
While the pCO2 responded exponentially to total suspended solids (TSS)
export when the TSS concentration was less than 100 kg m−3, it
decreased slightly and remained stable if the TSS concentration exceeded
100 kg m−3. This stable pCO2 is largely due to gully erosion that
mobilizes subsoils characterized by low organic carbon for decomposition. In
addition, human activities have changed the pCO2 dynamics. Particularly,
flow regulation by dams can diversely affect the temporal changes of
pCO2, depending on the physiochemical properties of the regulated waters
and adopted operation scheme. Given the high pCO2 in the Yellow River
waters, large potential for CO2 evasion is expected and warrants
further investigation. |
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