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Titel |
Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China |
VerfasserIn |
W. Xu, X. S. Luo, Y. P. Pan, L. Zhang, A. H. Tang, J. L. Shen, Y. Zhang, K. H. Li, Q. H. Wu, D. W. Yang, Y. Y. Zhang, J. Xue, W. Q. Li, Q. Q. Li, L. Tang, S. H. Lu, T. Liang, Y. A. Tong, P. Liu, Q. Zhang, Z. Q. Xiong, X. J. Shi, L. H. Wu, W. Q. Shi, K. Tian, X. H. Zhong, K. Shi, Q. Y. Tang, L. J. Zhang, J. L. Huang, C. E. He, F. H. Kuang, B. Zhu, H. Liu, X. Jin, Y. J. Xin, X. K. Shi, E. Z. Du, A. J. Dore, S. Tang, J. L. Collett, K. Goulding, Y. X. Sun, J. Ren, F. S. Zhang, X. J. Liu |
Medientyp |
Artikel
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Sprache |
Englisch
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ISSN |
1680-7316
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Digitales Dokument |
URL |
Erschienen |
In: Atmospheric Chemistry and Physics ; 15, no. 21 ; Nr. 15, no. 21 (2015-11-09), S.12345-12360 |
Datensatznummer |
250120146
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Publikation (Nr.) |
copernicus.org/acp-15-12345-2015.pdf |
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Zusammenfassung |
A Nationwide Nitrogen Deposition Monitoring Network (NNDMN)
containing 43 monitoring sites was established in China to measure
gaseous NH3, NO2, and HNO3 and particulate NH4+ and
NO3− in air and/or precipitation from 2010 to 2014. Wet/bulk
deposition fluxes of Nr species were collected by precipitation
gauge method and measured by continuous-flow analyzer; dry deposition fluxes
were estimated using airborne concentration measurements and inferential
models. Our observations reveal large spatial variations of atmospheric
Nr concentrations and dry and wet/bulk Nr deposition. On
a national basis, the annual average concentrations
(1.3–47.0 μg N m−3) and dry plus wet/bulk deposition fluxes
(2.9–83.3 kg N ha−1 yr−1) of inorganic Nr species
are ranked by land use as urban > rural > background sites and by regions
as north China > southeast China > southwest China > northeast
China > northwest China > Tibetan Plateau, reflecting the impact of
anthropogenic Nr emission. Average dry and wet/bulk N deposition
fluxes were 20.6 ± 11.2 (mean ± standard deviation) and
19.3 ± 9.2 kg N ha−1 yr−1 across China, with reduced N
deposition dominating both dry and wet/bulk deposition. Our results suggest
atmospheric dry N deposition is equally important to wet/bulk N deposition at
the national scale. Therefore, both deposition forms should be included when
considering the impacts of N deposition on environment and ecosystem health. |
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