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| Titel |
Spatial distribution of mercury deposition fluxes in Wanshan Hg mining area, Guizhou province, China |
| VerfasserIn |
Z. H. Dai, X. B. Feng, J. Sommar, P. Li, X. W. Fu |
| Medientyp |
Artikel
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| Sprache |
Englisch
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| ISSN |
1680-7316
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| Digitales Dokument |
URL |
| Erschienen |
In: Atmospheric Chemistry and Physics ; 12, no. 14 ; Nr. 12, no. 14 (2012-07-18), S.6207-6218 |
| Datensatznummer |
250011323
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| Publikation (Nr.) |
 copernicus.org/acp-12-6207-2012.pdf |
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| Zusammenfassung |
| The legacy of long-term mining activities in Wanshan mercury (Hg) mining
area (WMMA), Guizhou, China including a series of environmental issues
related to Hg pollution. The spatial distribution of gaseous elemental
mercury (Hg0) concentrations in ambient air were monitored using a
mobile RA-915+ Zeeman Mercury Analyzer during daytime and night time in
May 2010. The data imply that calcines and mine wastes piles located at
Dashuixi and on-going artisanal Hg mining activities at Supeng were major
sources of atmospheric mercury in WMMA. For a full year (May 2010 to May
2011), sampling of precipitation and throughfall were conducted on a weekly
basis at three sites (Shenchong, Dashuixi, and Supeng) within WMMA. Hg in
deposition was characterized by analysis of total Hg (THg) and dissolved Hg
(DHg) concentrations. The corresponding data exhibit a high degree of
variability, both temporarily and spatially. The volume-weighted mean THg
concentrations in precipitation and throughfall samples were 502.6 ng l−1
and 977.8 ng l−1 at Shenchong, 814.1 ng l−1and 3392.1 ng l−1
at Dashuixi, 7490.1 ng l−1and 9641.5 ng l−1 at Supeng,
respectively. THg was enhanced in throughfall compared to wet deposition
samples by up to a factor of 7. The annual wet Hg deposition fluxes were
29.1, 68.8 and 593.1 μg m−2 yr−1 at Shenchong, Dashuixi and
Supeng, respectively, while the annual dry Hg deposition fluxes were
estimated to be 378.9, 2613.6 and 6178 μg m−2 yr−1 at these
sites, respectively. Dry deposition played a dominant role in total
atmospheric Hg deposition in WMMA since the dry deposition fluxes were 10.4–37.9 times higher than the wet deposition fluxes during the whole sample
period. Our data showed that air deposition was still an important pathway
of Hg contamination to the local environment in WMMA. |
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