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Titel Ground-based remote sensing of volcanic CO2 and correlated SO2, HF, HCl, and BrO, in safe-distance from the crater
VerfasserIn André Butz, Anna Solvejg Dinger, Nicole Bobrowski, Julian Kostinek, Lukas Fieber, Constanze Fischerkeller, Giovanni Bruno Giuffrida, Frank Hase, Friedrich Klappenbach, Jonas Kuhn, Peter Lübcke, Lukas Tirpitz, Qiansi Tu
Konferenz EGU General Assembly 2017
Medientyp Artikel
Sprache en
Digitales Dokument PDF
Erschienen In: GRA - Volume 19 (2017)
Datensatznummer 250142967
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2017-6652.pdf
 
Zusammenfassung
Remote sensing of CO2 enhancements in volcanic plumes can be a tool to estimate volcanic CO2 emissions and thereby, to gain insight into the geological carbon cycle and into volcano interior processes. However, remote sensing of the volcanic CO2 is challenged by the large atmospheric background concentrations masking the minute volcanic signal. Here, we report on a demonstrator study conducted in September 2015 at Mt. Etna on Sicily, where we deployed an EM27/SUN Fourier Transform Spectrometer together with a UV spectrometer on a mobile remote sensing platform. The spectrometers were operated in direct-sun viewing geometry collecting cross-sectional scans of solar absorption spectra through the volcanic plume by operating the platform in stop-and-go patterns in 5 to 10 kilometers distance from the crater region. We successfully detected correlated intra-plume enhancements of CO2 and volcanic SO2, HF, HCl, and BrO. The path-integrated volcanic CO2 enhancements amounted to about 0.5 ppm (on top of the ∼400 ppm background). Key to successful detection of volcanic CO2 was A) the simultaneous observation of the O2 total column which allowed for correcting changes in the CO2 column caused by changes in observer altitude and B) the simultaneous measurement of volcanic species co-emitted with CO2 which allowed for discriminating intra-plume and extra-plume observations. The latter were used for subtracting the atmospheric CO2 background. The field study suggests that our remote sensing observatory is a candidate technique for volcano monitoring in safe distance from the crater region.