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Titel Monsoon-related transport processes: HCFC-22 as a tracer for East-Asian pollution transport
VerfasserIn Gabriele Stiller, Thomas von Clarmann, Sylvia Kellmann, Maksym Chirkov, Bärbel Vogel, Rolf Müller
Konferenz EGU General Assembly 2016
Medientyp Artikel
Sprache en
Digitales Dokument PDF
Erschienen In: GRA - Volume 18 (2016)
Datensatznummer 250128011
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2016-7951.pdf
 
Zusammenfassung
East-Asian pollution from Southern China or India was shown to be uplifted effectively by the Asian monsoon system to levels just below the tropopause. HCFC-22 nowadays has it strongest source region within East Asia. Due to its long lifetime in the troposphere, it is a very well suited transport tracer. We compare observations from MIPAS/Envisat of HCFC-22 with results from pollution transport modelling by the Lagrangian chemistry-transport model CLaMS. We find that East Asian pollution (and HCFC-22) is uplifted into the Asian monsoon anticyclone at the Eastern flank of the monsoon system. However, we do not find any indication of a significant transport through the tropopause of the Asian monsoon anticyclone into the stratosphere. In contrast, HCFC-22 is transported southwards into the tropics during the end phase and the break-down of the Asian monsoon anticyclone and distributed zonally in the tropics. By this a maximum layer of HCFC-22 just below the tropical tropopause is formed. Further transport into the stratosphere happens mainly by uplift within the upwelling branch of the Brewer-Dobson circulation.