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Titel Atmospheric organic aerosols in the Indo-Gangetic Plain: A synthesis
VerfasserIn Manmohan Sarin, Prashant Rajput
Konferenz EGU General Assembly 2016
Medientyp Artikel
Sprache en
Digitales Dokument PDF
Erschienen In: GRA - Volume 18 (2016)
Datensatznummer 250126121
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2016-5801.pdf
 
Zusammenfassung
Large-scale dispersal of atmospheric pollutants from biomass burning emissions (BBEs) and fossil-fuel combustion (FFc) sources in the Indo-Gangetic Plain (IGP); and a thick layer of haze advecting to the Bay of Bengal (BoB) is a conspicuous seasonal feature under favourable meteorological conditions during the wintertime (December-March). Our sustained studies in the source region of north-west-IGP have provided significant new understanding based on diagnostic ratios of OC/EC (10±2), WSOC/OC (0.52±0.02), nss-K+/OC (0.60±0.03) and ∑ PAHs/EC (1.3±0.2 mg/g) emitted from agricultural-waste (paddy-residue) burning in October-November that are significantly different from FFc sources. On average, organic aerosols account for ∼ 63 % and inorganic species about 23 % of PM2.5; whereas abundance of EC is no more than 4 %. Therefore, scattering species (organic and inorganic) have dominant impact on regional atmospheric chemistry and radiative forcing due to aerosols. The mass absorption efficiency (MAE) of EC (3.8±1.3 m2 g−1) exhibits significant decrease with increase in the concentrations of OC, nss-SO42− and NO3−. A scatter-plot for OC/EC and nss-SO42−/EC characteristically differentiates biomass burning emissions in the IGP than those from FFc sources in south-east Asia. Likewise, cross-plot of PAHs-isomers serve as potential tracers for BBEs in the IGP. Results emerging from these studies have major implications to re-assessment of model parameters for atmospheric radiative forcing due to black carbon from BBEs in the IGP, along the foot-hills of Himalaya and downwind marine atmospheric boundary layer over the Indian Ocean. Please fill in your abstract text.