 |
| Titel |
Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe |
| VerfasserIn |
C. Vigouroux, T. Blumenstock, M. Coffey, Q. Errera, O. García, N. B. Jones, J. W. Hannigan, F. Hase, B. Liley, E. Mahieu, J. Mellqvist, J. Notholt, M. Palm, G. Persson, M. Schneider, C. Servais, D. Smale, L. Thölix, M. De Mazière |
| Medientyp |
Artikel
|
| Sprache |
Englisch
|
| ISSN |
1680-7316
|
| Digitales Dokument |
URL |
| Erschienen |
In: Atmospheric Chemistry and Physics ; 15, no. 6 ; Nr. 15, no. 6 (2015-03-16), S.2915-2933 |
| Datensatznummer |
250119550
|
| Publikation (Nr.) |
 copernicus.org/acp-15-2915-2015.pdf |
|
|
|
|
|
| Zusammenfassung |
Ground-based Fourier transform infrared (FTIR) measurements of solar
absorption spectra can provide ozone total columns with a precision of
2% but also independent partial column amounts in about four
vertical layers, one in the troposphere and three in the stratosphere up to
about 45km, with a precision of 5–6%. We use eight of the
Network for the Detection of Atmospheric Composition Change (NDACC) stations
having a long-term time series of FTIR ozone measurements to study the total
and vertical ozone trends and variability, namely, Ny-Ålesund
(79° N), Thule (77° N), Kiruna (68° N), Harestua
(60° N), Jungfraujoch (47° N), Izaña (28° N),
Wollongong (34° S) and Lauder (45° S). The length of the
FTIR time series varies by station but is typically from about 1995 to
present. We applied to the monthly means of the ozone total and four partial
columns a stepwise multiple regression model including the following proxies:
solar cycle, quasi-biennial oscillation (QBO), El Niño–Southern Oscillation
(ENSO), Arctic and Antarctic Oscillation (AO/AAO), tropopause pressure (TP),
equivalent latitude (EL), Eliassen–Palm flux (EPF), and volume of polar
stratospheric clouds (VPSC).
At the Arctic stations, the trends are found mostly negative in the troposphere and
lower stratosphere, very mixed in the middle stratosphere, positive in the upper stratosphere
due to a large increase in the 1995–2003 period, and non-significant when considering the
total columns. The trends for mid-latitude and subtropical stations are all non-significant,
except at Lauder in the troposphere and upper stratosphere and at Wollongong for the total
columns and the lower and middle stratospheric columns where they are found positive. At
Jungfraujoch, the upper stratospheric trend is close to significance (+0.9 ± 1.0% decade−1).
Therefore, some signs of the onset of ozone mid-latitude recovery are observed only in the
Southern Hemisphere, while a few more years seem to be needed to observe it at the
northern mid-latitude station. |
| |
|
| Teil von |
|
|
|
|
|
|
|
|