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| Titel |
Trend and variability in ozone in the tropical lower stratosphere over 2.5 solar cycles observed by SAGE II and OSIRIS |
| VerfasserIn |
C. E. Sioris, C. A. McLinden, V. E. Fioletov, C. Adams, J. M. Zawodny, A. E. Bourassa, C. Z. Roth, D. A. Degenstein |
| Medientyp |
Artikel
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| Sprache |
Englisch
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| ISSN |
1680-7316
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| Digitales Dokument |
URL |
| Erschienen |
In: Atmospheric Chemistry and Physics ; 14, no. 7 ; Nr. 14, no. 7 (2014-04-07), S.3479-3496 |
| Datensatznummer |
250118569
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| Publikation (Nr.) |
 copernicus.org/acp-14-3479-2014.pdf |
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| Zusammenfassung |
| We have extended the satellite-based ozone anomaly time series to the
present (December 2012) by merging SAGE II (Stratospheric Aerosol and Gas Experiment
II) with OSIRIS (Optical Spectrograph and Infrared Imager System)
and correcting for the small bias (~0.5%) between them,
determined using their temporal overlap of 4 years. Analysis of the merged
data set (1984–2012) shows a statistically significant negative trend at all
altitudes in the 18–25 km range, including a trend of (−4.6 ± 2.6)% decade−1
at 19.5 km where the relative standard error is a minimum. We are
also able to replicate previously reported decadal trends in the tropical
lower-stratospheric ozone anomaly based on SAGE II observations.
Uncertainties are smaller on the merged trend than the SAGE II trend at all
altitudes. Underlying strong fluctuations in ozone anomaly due to El Niño–Southern Oscillation (ENSO), the altitude-dependent quasi-biennial
oscillation, and tropopause pressure need to be taken into account to reduce
trend uncertainties and, in the case of ENSO, to accurately determine the
linear trend just above the tropopause. We also compare the observed ozone
trend with a calculated trend that uses information on tropical upwelling
and its temporal trend from model simulations, tropopause pressure trend
information derived from reanalysis data, and vertical profiles from SAGE II
and OSIRIS to determine the vertical gradient of ozone and its trend. We
show that the observed trend agrees with the calculated trend and that the
magnitude of the calculated trend is dominated by increased tropical
upwelling, with minor but increasing contribution from the vertical ozone
gradient trend as the tropical tropopause is approached. Improvements are
suggested for future regression modelling efforts which could reduce trend
uncertainties and biases in trend magnitudes, thereby allowing accurate
trend detection to extend below 18 km. |
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