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Titel |
Estimation of the SO2 source term for the Holuhraun event and its influence on central Europe air quality |
VerfasserIn |
Delia Arnold, Nina Iren Kristiansen, Nicolas Theys, Hugues Brenot, Christian Maurer, Gerhard Wotawa, Kerstin Stebel, Robert Holla, Stefan Gilge, Johannes Flemming, Andreas Stohl, Marcus Hirtl |
Konferenz |
EGU General Assembly 2015
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Medientyp |
Artikel
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Sprache |
Englisch
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Digitales Dokument |
PDF |
Erschienen |
In: GRA - Volume 17 (2015) |
Datensatznummer |
250110080
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Publikation (Nr.) |
EGU/EGU2015-10044.pdf |
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Zusammenfassung |
On 29 August 2014 a fissure eruption began in Holuhraun, Northeastern Iceland, associated with increased volcanic activity in the Bárdarbunga system. For more than 150 days, the eruption released large quantities of SO2 into the atmosphere affecting not only the local Icelandic air quality, but also leading to periods of increased ambient SO2 concentrations in parts of mainland Europe. During the second half of September, significant amounts of SO2 were rapidly transported southward by favourable meteorological conditions and several countries in Central Europe experienced high ground-level SO2 concentrations. The measured concentrations reached and even exceeded the EC directive health thresholds.
In this work, we evaluate the air quality effects in Europe during this targeted period using both ground-based and satellite observations (GOME2B and OMI) as well as dispersion modelling with the Lagrangian particle model FLEXPART. We estimate the volcanic SO2 source emissions by comparing the satellite observations with atmospheric transport model simulations in an inverse modelling approach. The estimated source term is evaluated against independent ground-based observational data (e.g. MAX-DOAS, Brewer) and used as emission term in dispersion model forecasts for evaluating the air quality effects in Europe. In addition, the potential use of air quality data to perform the source term estimation by inversion with ground-based data will also be investigated. |
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