dot
Detailansicht
Katalogkarte GBA
Katalogkarte ISBD
Suche präzisieren
Drucken
Download RIS
Hier klicken, um den Treffer aus der Auswahl zu entfernen
Titel Formation and growth rates of atmospheric nanoparticles: four years of observations at two West Siberian stations
VerfasserIn Mikhail Yu. Arshinov, Boris D. Belan, Denis K. Davydov, Artem V. Kozlov, Victoria Arshinova
Konferenz EGU General Assembly 2015
Medientyp Artikel
Sprache Englisch
Digitales Dokument PDF
Erschienen In: GRA - Volume 17 (2015)
Datensatznummer 250105245
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2015-4723.pdf
 
Zusammenfassung
In spite of fact that the first report on the new particle formation (NPF) itself was done by John Aitken more than one century ago (Aitken, 1898), a phenomenon of NPF bursts taken place in the atmosphere was discovered not very long ago. Nevertheless, to date it is known that they may occur quite often in a variety of environments (Kulmala et al., 2004; Hirsikko et al., 2011). Siberia occupies a vast area covered by forests, but the comprehensive data on burst frequency, as well as on formation and growth rates of freshly nucleated particles in this key region are still lacking. Continuous measurements of aerosol size distribution carried out in recent years at two West Siberian stations (TOR-station – 56o28’41"N, 85o03’15"E; Fonovaya Observatory – 56o25’07"N, 84o04’27"E) allowed this gap in data to be filled up. Analysis of the size spectra classified in accordance with criteria proposed by Dal Maso et al. (2005) and Hammed et al. (2007) enabled a conclusion to be drawn that NPF events in Wets Siberia are more often observed during spring (from March to May) and early autumn (secondary frequency peak in September). On average, particle formation bursts took place on 23-28Â% of all days. Such a seasonal pattern of the NPF occurrence is very similar to one observed at SMEAR II Station (Hyytiälä, Finland; DalÂMaso et al. 2005, 2007). Formation rates (FR) of particles with diameters below 25 nm varied in a wide range from 0.1 to 10 cm-3 s-1. Mean values of FR for the entire period of observations were 1.7 cm-3s-1 (median = 1.13 cm-3 s-1) at TOR-station and 0.88 cm-3 s-1 (median = 0.69 cm-3 s-1) at Fonovaya Observatory. Enhanced values of FR are usually observed from spring to autumn. Mean growth rates of observed at TOR-station and Fonovaya Observatory were 6.5 nm h-1 (median = 5.0 nm h-1) and 8.3 nm h-1 (median = 6.4 nm h-1), respectively. This work was supported by the Branch of Geology, Geophysics and Mining Sciences of RAS (ProgramÂNo. 5); State contracts of the Ministry of Education and Science of Russia No. 14.604.21.0100, (RFMTFIBBB210290) and No. 14.613.21.0013 (RFMEFI61314X0013); and Russian Foundation for Basic Research (grant No. 14-05-00590). Dal Maso, M., Kulmala, M., Riipinen, I., Wagner, R., Hussein, T., Aalto, P. P., and Lehtinen, K. E. J. (2005). Formation and growth of fresh atmospheric aerosols: eight years of aerosol size distribution data from SMEAR II, Hyytiälä, Finland, Boreal Environ. Res. 10, 323–336. Dal Maso, M., Sogacheva, L., Aalto, P., Riipinen, I., Komppula, M., Tunved, P., Korhonen, L., Suur-uski, V., Hirsikko, A., Kurten, T., Kerminen, V., Lihavainen, H., Viisanen, Y., Hansson, H., and Kulmala, M. (2007). Aerosol size distribution measurements at four Nordic field stations: identification, analysis and trajectories analysis of new particle formation bursts, Tellus B 59, 350–361. Hamed,ÂA., Joutsensaari,ÂJ., Mikkonen,ÂS., Sogacheva,ÂL., DalÂMaso,ÂM., Kulmala,ÂM., CavalliÂF., FuzziÂS., Facchini,ÂM.ÂC., Decesari,ÂS., Mircea,ÂM., Lehtinen,ÂK.ÂE.ÂJ., and Laaksonen,ÂA. (2007). Nucleation and growth of new particles in Po Valley, Italy, Atmos. Chem. Phys. 7, 355–376. Hirsikko,ÂA., Nieminen,ÂT., Gagné,ÂS., Lehtipalo,ÂK., Manninen,ÂH.ÂE., Ehn,ÂM., Hõrrak,ÂU., Kerminen,ÂV.-M., Laakso,ÂL., McMurry,ÂP.ÂH., Mirme,ÂA., Mirme,ÂS., Petäjä,ÂT., Tammet,ÂH., Vakkari,ÂV., Vana,ÂM., and Kulmala,ÂM. (2011). Atmospheric ions and nucleation: a review of observations, Atmos. Chem. Phys. 11, 767–798. Kulmala, M., Vehkamäki, H., Petäjä, T., Dal Maso, M., Lauri A., Kerminen, V.-M., Birmili, W., and McMurry, P. H. (2004a) Formation and growth rates of ultrafine atmospheric particles: a review of observations, J. Aerosol ScienceÂ35, 143–176.