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Titel On the feasibility of cirrus cloud thinning: Dependence of homo- and heterogeneous ice nucleation on latitude and season
VerfasserIn David Mitchell, Anne Garnier, Melody Avery
Konferenz EGU General Assembly 2015
Medientyp Artikel
Sprache Englisch
Digitales Dokument PDF
Erschienen In: GRA - Volume 17 (2015)
Datensatznummer 250103133
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2015-2532.pdf
 
Zusammenfassung
While GCM testing of cirrus cloud climate engineering (CE) reveals some advantages over stratospheric aerosol injection, cirrus CE will not work when ice is primarily formed through heterogeneous nucleation for T < -38°C. Field campaigns have shown that ice in cold cirrus is generally produced heterogeneously, but these campaigns have not addressed the cirrus at high latitudes that would determine the effectiveness of cirrus CE. This presentation introduces a new understanding of the satellite retrieved “effective absorption optical depth ratio”, or βeff, based on the 12.05 and 10.60 μm channels of the imaging infrared radiometer (IIR) aboard the CALIPSO satellite. Using βeff calculations from in situ data, it is found that βeff is tightly related to the N/IWC ratio, where N = ice particle number concentration and IWC = ice water content. This is because N is primarily determined by the smallest ice particles, and βeff is primarily due to differences in wave resonance (i.e. photon tunneling) absorption, a process that is only significant when ice particle maximum dimension D < ~ 60 μm (i.e. when wavelength and effective particle size are comparable). Thus βeff is a measure of the concentration of small (D < 60 μm) ice crystals relative to the concentration of larger ice particles. Since homogeneous ice nucleation generally results in N > 500 liter-1, with a relatively high concentration of small ice crystals, βeff may be used to determine when homogeneous nucleation dominates in a region for T < -38°C. Satellite retrievals of βeff from anvil cirrus having N > 500 liter-1 (based on co-located/coincident in situ measurements) suggest that homogeneous nucleation dominates when βeff > 1.15 ± 0.05. A global analysis of βeff was conducted for the boreal summer (July-Aug.) and winter (Jan.-Feb.) of 2007 and 2008, respectively. Using βeff to discriminate between regions of homo- and heterogeneous ice nucleation for cirrus clouds having emissivities between 0.4 and 0.7 and T < -38°C, our preliminary results suggest that homogeneous ice nucleation is very common during the winter months at high latitudes. This is consistent with GCM predicted concentrations of mineral dust at 200 hPa, which are minimal during winter at high latitudes. Regarding cirrus CE, it was recently shown that seeding only 15% of the globe with the highest solar noon zenith angles at any given time (i.e. the high latitudes during late fall-winter-spring) produced a mean global cooling of 1.4°K, with much stronger cooling at high latitudes. Our preliminary findings suggest that homogeneous ice nucleation may dominate in winter at high latitudes, a necessary condition for this seeding strategy to be viable.