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Titel Comparisons between satellite-derived datasets of stratospheric NOy species: using a photochemical model to account for diurnal variations
VerfasserIn Patrick Sheese, Kaley Walker, Chris McLinden, Chris Boone, Peter Bernath, John Burrows, Bernd Funke, Didier Fussen, Gloria Manney, Donal Murtagh, Cora Randall, Piera Raspollini, Alexei Rozanov, James Russell, Jo Urban, Thomas von Clarmann, Joseph Zawodny
Konferenz EGU General Assembly 2014
Medientyp Artikel
Sprache Englisch
Digitales Dokument PDF
Erschienen In: GRA - Volume 16 (2014)
Datensatznummer 250099970
Publikation (Nr.) Volltext-Dokument vorhandenEGU/EGU2014-15829.pdf
 
Zusammenfassung
The ACE-FTS (Atmospheric Chemistry Experiment – Fourier Transform Spectrometer) instrument on the Canadian satellite SCISAT, which has been in operation now for over 10 years, has the capability of deriving stratospheric profiles of many of the NOy (NO + NO2+ NO3+ 2xN2O5+ HNO3+ HNO4+ ClONO2+ BrONO2) species. However, as a solar occultation instrument, opportunities for ACE-FTS and another given satellite instrument to observe a common air mass, can be rather limited. In the case of comparing species that exhibit significant diurnal variation, finding “coincident” measurements can be even more difficult. In order for the measurements to be considered common-volume, the required difference between measurement times can be limitingly small. In this study, for each ACE-FTS measurement, we use a photochemical box model to simulate the diurnal variations of different NOy species over that day. The ACE-FTS NOy profiles are then scaled to the local times of coincident measurements from different satellite instruments—GOMOS, MIPAS, MLS, OSIRIS, POAM III, SAGE III, SCIAMACHY, and SMR. This allows for a much larger number of coincidences to be utilized. This study will discuss the advantages and limitations of this technique, as well as the results from comparing NO, NO2, N2O5, HNO3, and ClONO2 between ACE-FTS and other atmospheric limb sounders.