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Titel MIPAS/ENVISAT observations of decay products of isoprene and other hydrocarbons in the upper troposphere and simulations with the new mechanism MIM3 in the CCM EMAC
VerfasserIn C. Brühl, D. Taraborrelli, T. von Clarmann, N. Glatthor, A. Wiegele, B. Funke
Konferenz EGU General Assembly 2012
Medientyp Artikel
Sprache Englisch
Digitales Dokument PDF
Erschienen In: GRA - Volume 14 (2012)
Datensatznummer 250069838
 
Zusammenfassung
Simultaneous limb observations of HCOOH, CO, PAN, C2H6, O3, NOx and other species by MIPAS in the upper troposphere and lower stratosphere are compared with results of the chemical circulation model EMAC. To allow for point by point comparisons with the satellite data, the tropospheric meteorology of the CCM is nudged by observations of ECMWF. The method is used for evaluation and further development of the new isoprene oxidation scheme MIM3 and also for checking and distinguishing biogenic and anthropogenic emissions used in the model. We show that the model is able to reproduce the main features of the observations, including the seasonal cycle, and that proper modelling of isoprene chemistry (and to less extent terpene chemistry) is critical for understanding the observed chemical composition of the upper troposphere.